This didn't, however, mark the beginning of a solo career, and although Haydee left the group in 1961 in order to live in the U.S., Omara continued singing with Cuarteto las d'Aida until 1967. In 1967 Portuondo embarked on a solo career, and in the same year represented Cuba at the Sopot Festival in Poland, singing Juanito Marquez' "Como un Milagro". Alongside her solo work, in the 1970s she sang with charanga band Orquestra Aragon, and toured with them both in the Communist and non-Communist worlds. In 1974 she recorded, with guitarist Martin Rojas, what would become one of her most critically acclaimed albums in which she sings praises to Salvador Allende and the people of Chile a year after the military coup led by General Augusto Pinochet. Among many other hits from the album, she also praises the work of Ernesto "Che" Guevara in the beautiful "Hasta Siempre". During the 1970s and 1980s Portuonda enjoyed considerable success at home and abroad, with tours, albums (including one of her most lauded recordings in 1984 with Adalberto Alvarez), film rôles, and her own television series. Her international profile was due to soar, however, in 1996. Portuondo sang (duetting with Compay Segundo) on the album Buena Vista Social Club in 1996.
This led, not only to more touring (including playing at Carnegie Hall with the Buena Vista troupe) and her appearance in Wim Wenders' film The Buena Vista Social Club, but to two further albums for the World Circuit label: Buena Vista Social Club Presents Omara Portuondo (2000) and Flor de Amor (2004). In July 2005 she presented a symphonic concert of her most important repertoire at the Berlin Festival Classic Open Air am Gendarmenmarkt for an audience of 7,000. The entire program was specially orchestrated by Roberto Sánchez Ferrer, a colleague with whom she had worked during her early years at Havana's Tropicana Club. Scott Lawton conducted the Deutsches Filmorchester Babelsberg.
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