Berns signed them to the United Artists label and wrote the hit, "Cry Baby" for them with songwriting partner Jerry Ragovoy. The song topped the R&B chart and went to #4 on the Billboard Hot 100 chart in 1963. It sold over one million copies, and was awarded a gold disc. Mimms and the group had a follow-up double sided hit, "For Your Precious Love" and "Baby Don't You Weep", both tracks entering the Billboard Top 30, before he went solo in 1964. In 1966, Berns and Ragavoy produced another big hit for Mimms, "I'll Take Good Care Of You", which climbed to #15 in the R&B chart and #30 in the Hot 100.
He worked with Jimi Hendrix in the UK the following year. He did some recording on the MGM and Verve labels. In 1969, Led Zeppelin performed an extended version of Mimms' "As Long As I have You" at various stops on their U.S tour. In the 1970s, he released a few funk songs as Garnet Mimms and the Truckin' Co. He had his only hit in the United Kingdom at this time, when "What It Is" reached number 44 for one week on the UK Singles Chart in June 1977. Mimms was given a Pioneer Award in 1999 by the Rhythm and Blues Foundation. In the 1980s, Garnet found his calling ministering to lost souls in prison, but in 2007, returned to recording and a year later, released a new gospel album Is Anybody Out There? on the Evidence label, produced and (primarily) written by Jon Tiven.
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